Biogeosciences Discuss., 10, 19935-19968, 2013
www.biogeosciences-discuss.net/10/19935/2013/
doi:10.5194/bgd-10-19935-2013
© Author(s) 2013. This work is distributed
under the Creative Commons Attribution 3.0 License.
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This discussion paper is under review for the journal Biogeosciences (BG).
The 129-Iodine content of subtropical Pacific waters: impact of Fukushima and other anthropogenic 129I sources
T. P. Guilderson1,2, S. J. Tumey1, T. A. Brown1, and K. O. Buesseler3
1Center for Accelerator Mass Spectrometry, Lawrence Livermore National Laboratory, Livermore CA, USA
2Department of Ocean Sciences and Institute of Marine Sciences, University of California, Santa Cruz, CA, USA
3Department of Marine Chemistry and Geochemistry, Woods Hole Oceanographic Institution, Woods Hole, MA, USA

Abstract. Results obtained from a dedicated radiochemistry cruise approximately 100 days after the 11 March 2011 Tohoku earthquake and subsequent disaster at the Dia'ichi Fukushima Nuclear Power Plant show that Fukushima derived radionuclides in the nearby ocean environment had penetrated, on average, to ≤250 m depth (1026.5 kg m−3 potential density surface). The excess inventory of Fukushima-derived 129I in the region (∼150 000 km2) sampled during the cruise is estimated to have been between 0.89 and 1.173 billion Bq (∼136 to ∼179 g) of 129I. Based on a tight tracer–tracer relation with 134Cs (or 137Cs) and estimates that most of the excess cesium is due to direct discharge, we infer that much of the excess 129I is from direct (non-atmospheric deposition) discharge. After taking into account oceanic transport, we estimate the direct discharge off Fukushima to have been ∼1 kg 129I. Although this small pulse is dwarfed by the ∼90 kg of weapons-testing derived 129I that was released into the environment in the late 1950s and early 1960s, it should be possible to use Fukushima derived 129I and other radionuclides (e.g., 134, 137Cs) to study transport and entrainment processes along the Kuroshio Current.

Citation: Guilderson, T. P., Tumey, S. J., Brown, T. A., and Buesseler, K. O.: The 129-Iodine content of subtropical Pacific waters: impact of Fukushima and other anthropogenic 129I sources, Biogeosciences Discuss., 10, 19935-19968, doi:10.5194/bgd-10-19935-2013, 2013.
 
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